Most design equations using an experimental regression are approximations, however, I would say that the 3-term equation is an even more loose approximation, because it takes experimental data, tries to fit a regression to it, and then adjusts the terms to make the analysis easier for the average engineer. If you are trying to increase stiffness by limiting capacity of a diaphragm with tight nail spacing, I don't know of a good way to do so offhand using the 3-term equation. However, if you artificially cap the diaphragm capacity below the nominally adjusted capacity in the relevant tables, I could see a way of increasing the stiffness of the system by reducing the nail slip value per nail and shear stiffness in the 4-term equation.
Long story short, if using the 4-term, I believe so, if using the 3-term and Ga, I don't know of a convenient way to increase stiffness.