That seems reasonable. When I worked in NVH we were very interested in finding sources of tonal problems, so I'd typically stick a mic in the engine compartment, or under the body, and hit everything in sight until I found a source of the right frequency.
Then we'd remove, modify, or cover that component and see if we had affected the noise. There are other ways to do this, but this one works, and you can do it by yourself.
Yes, we would often compare FRFs with sound spectrums, in the engine noise lab this was an important part of our source identification technique, since that tells you a lot about the radiation efficiency of each component.
It sounds like you are on the right track. Cheers
Greg Locock