I would have thought that you would need a valve for isolating the new coolers from the existing units and could use this valve to “tune” the system. Basically I agree with Plainwater that you need a pump with a bigger capacity because your existing coolers have so much friction as equivalent to the shutoff head of the pump. That friction will not diminish unless you accept a lower flow to the cooler.
If you fit the additional coolers, with a valve as suggested, you can turn the valve until the combined friction loss of the valve and the new coolers matches the friction loss of the existing units. Then your pump will operate same as before and each cooler should receive nearly identical flow. Mind you the total flow has not been increased. If you open the valve fully, as though the new coolers have been fitted without the valve, more water will pass into the new coolers leaving the existing coolers starved of water.
You can play around with the valve to vary the flows in the cooler but you are not going to get more flow out of your pump unless the total resistance is reduced.
Calculation is possible as described by rbculter but you need to have a fairly good idea of the friction characteristic. Both the pump curve and the system characteristic (combined friction losses + any static lift) obeys the H=KQ*Q (H=head, Q=discharge, K=constant) and you can plot the two out. The crossing point of the two curves is your operating point. My suggested valve, equivalent to your pressure regulator idea, simply gives a means to vary the K value of your system characteristic. A quick way to appreciate your problem is treat K1=200/(60*60)=1/18 as your existing system. The new cooler will have K2=150/(30*30)=1/6. If you combined the two together then the combined K=1/18+1/6 = 2/9. Plot these graphs in an Excel spreadsheet and superimpose them with you pump curve (x=Q, y=H). You will see your pump is not man enough to do the trick you have got in mind.